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Journal Articles

Experimental investigation on local flow structures of upward cap-bubbly flows in a vertical large-size square channel

Sun, Haomin; Kunugi, Tomoaki*; Yokomine, Takehiko*; Shen, X.*; Hibiki, Takashi*

Experimental Thermal and Fluid Science, 154, p.111171_1 - 111171_24, 2024/05

 Times Cited Count:0

JAEA Reports

Assessment of probability of aircraft crashes for Nuclear Science Research Institute

Kamikawa, Yutaka; Suzuki, Makoto; Agake, Toshiki; Murakami, Takahiko; Morita, Yusuke; Shiina, Hidenori; Fukushima, Manabu; Hirane, Nobuhiko; Ouchi, Yasuhiro

JAEA-Technology 2023-030, 57 Pages, 2024/03

JAEA-Technology-2023-030.pdf:1.93MB

Owing to the publication of the latest data about aircraft crashes by Nuclear Regulation Authority (NRA), it was necessary to re-evaluate the probabilities of aircraft crashes for Nuclear Science Research Institute (NSRI). By using of the assessment method provided in "Regulatory Guide of the Assessment Standard for Probability of Airplane Crash on a Nuclear Power Reactor Facility", we re-evaluated the probabilities of aircraft crashes against the nuclear facilities in NSRI. As a result of the evaluations, the sum of the probabilities of aircraft crashes against Waste Treatment Facilities (maximum probability among all nuclear facilities in NSRI) is 5.68$$times$$10$$^{-8}$$ (times/(reactor $$cdot$$ year)) which is lower than 10$$^{-7}$$ (times/(reactor $$cdot$$ year)) that is the assessment criterion whether aircraft crashes is considered to be "anticipated external human induced events" in design basis or not.

Journal Articles

Evaluation of excavation damaged zones (EDZs) in Horonobe Underground Research Laboratory (URL)

Hata, Koji*; Niunoya, Sumio*; Aoyagi, Kazuhei; Miyara, Nobukatsu*

Journal of Rock Mechanics and Geotechnical Engineering, 16(2), p.365 - 378, 2024/02

Excavation of underground caverns, such as mountain tunnels and energy-storage caverns, may cause the damages to the surrounding rock as a result of the stress redistribution. In this influenced zone, new cracks and discontinuities are created or propagate in the rock mass. Therefore, it is effective to measure and evaluate the acoustic emission (AE) events generated by the rocks, which is a small elastic vibration, and permeability change. The authors have developed a long-term measurement device that incorporates an optical AE (O-AE) sensor, an optical pore pressure sensor, and an optical temperature sensor in a single multi-optical measurement probe (MOP). Japan Atomic Energy Agency has been conducting R&D activities to enhance the reliability of high-level radioactive waste (HLW) deep geological disposal technology. In a high-level radioactive disposal project, one of the challenges is the development of methods for long-term monitoring of rock mass behavior. Therefore, in January 2014, the long-term measurements of the hydro-mechanical behavior of the rock mass were launched using the developed MOP in the vicinity of 350 m below the surface at the Horonobe Underground Research Center. The measurement results show that AEs occur frequently up to 1.5 m from the wall during excavation. In addition, hydraulic conductivity increased by 2 to 4 orders of magnitude. Elastoplastic analysis revealed that the hydraulic behavior of the rock mass affected the pore pressure fluctuations and caused micro-fractures. Based on this, a conceptual model is developed to represent the excavation damaged zone (EDZ), which contributes to the safe geological disposal of radioactive waste.

Journal Articles

Understanding muon diffusion in perovskite oxides below room temperature based on harmonic transition state theory

Ito, Takashi; Higemoto, Wataru; Shimomura, Koichiro*

Physical Review B, 108(22), p.224301_1 - 224301_11, 2023/12

 Times Cited Count:1 Percentile:0(Materials Science, Multidisciplinary)

Journal Articles

Multi-dimensional characteristics of upward bubbly flows in a vertical large-size square channel

Sun, Haomin; Kunugi, Tomoaki*; Yokomine, Takehiko*; Shen, X.*; Hibiki, Takashi*

International Journal of Heat and Mass Transfer, 211, p.124214_1 - 124214_17, 2023/09

 Times Cited Count:2 Percentile:53.66(Thermodynamics)

Journal Articles

Local electronic structure of interstitial hydrogen in MgH$$_2$$ inferred from muon study

Kadono, Ryosuke*; Hiraishi, Masatoshi*; Okabe, Hirotaka*; Koda, Akihiro*; Ito, Takashi

Journal of Physics; Condensed Matter, 35(28), p.285503_1 - 285503_13, 2023/07

 Times Cited Count:0 Percentile:0(Physics, Condensed Matter)

Journal Articles

Effectiveness evaluation methodology of the measures for improving resilience of nuclear structures at ultra-high temperature

Onoda, Yuichi; Kurisaka, Kenichi; Yamano, Hidemasa

Proceedings of 30th International Conference on Nuclear Engineering (ICONE30) (Internet), 7 Pages, 2023/05

The objective of this study is to develop an effectiveness evaluation methodology of the measures for improving resilience of nuclear structures at ultra-high temperature by using the failure mitigation technology. At the beginning, to identify the accident sequences having the potential to improve resilience, the characteristics of a next-generation loop-type sodium-cooled fast reactor (SFR) in Japan has been investigated by analyzing the event tree of level-1 and level-2 probabilistic risk assessment. As a result, event sequences of loss of heat removal systems (LOHRS) are identified. The effectiveness of the measures for improving resilience is evaluated by quantifying the reduction rate of core damage frequency before and after the introduction of the measures for improving resilience for all the accident sequences leading to LOHRS. To examine applicability of the developed methodology, a trial evaluation has conducted for a next-generation loop-type SFR in Japan. Through the applicability examined, the method for the effectiveness evaluation was developed successfully. The refinement of the conditional success probability of the measures for improving resilience is the future work.

Journal Articles

New approach to understanding the experimental $$^{133}$$Cs NMR chemical shift of clay minerals via machine learning and DFT-GIPAW calculations

Okubo, Takahiro*; Takei, Akihiro*; Tachi, Yukio; Fukatsu, Yuta; Deguchi, Kenzo*; Oki, Shinobu*; Shimizu, Tadashi*

Journal of Physical Chemistry A, 127(4), p.973 - 986, 2023/02

 Times Cited Count:1 Percentile:50.66(Chemistry, Physical)

The identification of adsorption sites of Cs on clay minerals has been studied in the fields of environmental chemistry. The nuclear magnetic resonance (NMR) experiments allow direct observations of the local structures of adsorbed Cs. The NMR parameters of $$^{133}$$Cs, derived from solid-state NMR experiments, are sensitive to the local neighboring structures of adsorbed Cs. However, determining the Cs positions from NMR data alone is difficult. This paper describes an approach for identifying the expected atomic positions of Cs adsorbed on clay minerals by combining machine learning (ML) with experimentally observed chemical shifts. A linear ridge regression model for ML is constructed from the smooth overlap of atomic positions descriptor and gauge-including projector augmented wave (GIPAW) ab initio data. The $$^{133}$$Cs chemical shifts can be instantaneously calculated from the Cs positions on any clay layers using ML. The inverse analysis from the ML model can derive the atomic positions from experimentally observed chemical shifts.

Journal Articles

Preliminary studies of XANES and DFT calculation of Ru extraction by imino-diacetamide and related compounds

Sasaki, Yuji; Nakase, Masahiko*; Kaneko, Masashi; Kobayashi, Toru; Takeshita, Kenji*; Matsumiya, Masahiko*

Analytical Sciences, 5 Pages, 2023/00

 Times Cited Count:0 Percentile:0(Chemistry, Analytical)

We conducted three field researches on Ru-extraction, XANES, and DFT-calculation. The order of the distribution ratio, D(Ru), from acid, HCl $$>$$ H$$_2$$SO$$_4$$ $$>$$ HNO$$_3$$ $$>$$ HClO$$_4$$, by MIDOA is studied by XANES spectra, which indicates the valency change of Ru in HCl media and supports the ion pairing extraction of anionic Ru ion and cationic MIDOA. The same extractant trend, NTAamide $$>$$ MIDOA $$>$$ IDOA, due to D values as the energy gap of HOMO and LUMO could be found by DFT calculation, which suggests that the reaction heat has a positive correlation with extractability for extractant.

Journal Articles

On the origin of localized electrons in SrTiO$$_3$$ metallized by hydrogen irradiation

Ito, Takashi

Meson, (56), p.21 - 26, 2022/09

no abstracts in English

JAEA Reports

Development of technology for rapid analysis of strontium-90 with low isotopic abundance using laser resonance ionization (Contract research); FY2020 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; The University of Tokyo*

JAEA-Review 2022-014, 106 Pages, 2022/08

JAEA-Review-2022-014.pdf:10.42MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2018, this report summarizes the research results of the "Development of technology for rapid analysis of strontium-90 with low isotopic abundance using laser resonance ionization" conducted from FY2018 to FY2021 (this contract was extended to FY2021). Since the final year of this proposal was FY2021, the results for four fiscal years were summarized. The present study aims to develop a rapid analysis technique for strontium-90 using diode laser-based resonance ionization with elemental and isotopic selectivity. Strontium-90 is one of the major difficult-to-measure nuclides released into the environment due to the accident at TEPCO's Fukushima Daiichi Nuclear Power Station.

Journal Articles

Hydrogen absorption and diffusion behaviors in cube-shaped palladium nanoparticles revealed by ambient-pressure X-ray photoelectron spectroscopy

Tang, J.*; Seo, O.*; Rivera Rocabado, D. S.*; Koitaya, Takanori*; Yamamoto, Susumu*; Namba, Yusuke*; Song, C.*; Kim, J.*; Yoshigoe, Akitaka; Koyama, Michihisa*; et al.

Applied Surface Science, 587, p.152797_1 - 152797_8, 2022/06

 Times Cited Count:7 Percentile:75.56(Chemistry, Physical)

The hydrogen absorption and diffusion mechanisms on cube-shaped Pd nanoparticles (NPs) which are important hydrogen-storage materials were studied using X-ray photoelectron spectroscopy and DFT calculations. In the surface region, hydrogen absorption showed almost similar behavior regardless of the NPs size. It was found that the octahedral sites are more favorable than the tetrahedral sites for hydrogen occupation. We also clarified that the hydrogen atoms absorbing on the smaller-sized Pd NPs diffuse to the subsurface more actively because of the weakened Pd-H bond by the surface disordering, which plays an important role in hydrogen adsorption at a low H$$_{2}$$ pressure.

Journal Articles

Flow regime and void fraction predictions in vertical rod bundle flow channels

Han, X.*; Shen, X.*; Yamamoto, Toshihiro*; Nakajima, Ken*; Sun, Haomin; Hibiki, Takashi*

International Journal of Heat and Mass Transfer, 178, p.121637_1 - 121637_24, 2021/10

 Times Cited Count:7 Percentile:57.51(Thermodynamics)

Journal Articles

Development of effectiveness evaluations technology of the measures for improving resilience of nuclear structures at ultra high temperature

Onoda, Yuichi; Nishino, Hiroyuki; Kurisaka, Kenichi; Yamano, Hidemasa

Proceedings of Asian Symposium on Risk Assessment and Management 2021 (ASRAM 2021) (Internet), 11 Pages, 2021/10

The effectiveness evaluations technology of the measures for improving resilience by applying a fracture control concept under ultra-high temperature conditions has developed for prototype sodium-cooled fast reactor Monju as a model plant, and the trial evaluation has conducted using this technology in this paper. The important accident sequences to which the fracture control concept is expected to be applied under ultra-high temperature condition are identified by investigating the results of the existing researches of level-2 probabilistic risk assessment for Monju. Accident sequences categorized in protected loss of heat sink and loss of reactor level are both identified as such important accident sequences which has the potential to prevent core damage. This study has developed the technology to evaluate the effectiveness of improving resilience, where the headings which stand for success or failure of the measures to improve resilience are introduced into the event tree, the branch probability of them is set, and the effectiveness of improving resilience is expressed as the reduction of core damage frequency. As a result of the trial evaluation of the effectiveness for the measures to improve resilience, it is confirmed that core damage frequency can be reduced by applying fracture control concept. The branch probability of the measures to improve resilience proposed in this study is tentatively assigned based on the assumption. This value is expected to be quantified by the forthcoming analyses of the integrity for the reactor vessel structure at ultra-high temperature. The technology developed in this study will be applied for the evaluation of improving resilience of the next generation sodium-cooled fast reactor.

Journal Articles

3D FEM soil-structure interaction analysis for Kashiwazaki-Kariwa Nuclear Power Plant considering soil separation and sliding

Ichihara, Yoshitaka*; Nakamura, Naohiro*; Moritani, Hiroshi*; Choi, B.; Nishida, Akemi

Frontiers in Built Environment (Internet), 7, p.676408_1 - 676408_14, 2021/06

The objective of this study is the improvement of response evaluations of structures, facilities and equipment in evaluation of three-dimensional seismic behavior of nuclear power plant facilities, by three-dimensional finite element method model, including separation and sliding between the soil and the basement walls. To achieve this, simulation analyses of Kashiwazaki Kariwa nuclear power plant unit 7 reactor building under the 2007 Niigataken-chuetsu-oki earthquake event were carried out. These simulation analyses consider soil-structure interaction using a three-dimensional finite element method model in which the soil and building are three-dimensionally modeled by the finite element method. It is found that basemat uplift is generated on east side of the basemat edge, and this has an important influence on the results. The importance is evidenced by the difference of local response in soil pressure characteristics beneath the edge of basemat, the soil pressure characteristics along the east side of basement wall and the maximum acceleration response at the west end of the embedded surface. Although, in this particular study, basemat uplift, separation and sliding have only a relatively small influence on the maximum acceleration response of embedded surface and the soil pressure characteristics along the basement walls and beneath the basemat, under strong earthquake motion, these influences can be significant, therefore appropriate evaluation of this effect should be considered.

Journal Articles

Kinetic and Fourier transform infrared studies on the thermal decomposition of sodium hydride

Kawaguchi, Munemichi

Journal of Physical Chemistry C, 125(22), p.11813 - 11819, 2021/06

 Times Cited Count:2 Percentile:13.34(Chemistry, Physical)

Isothermal and constant heating thermogravimetry-differential thermal analysis (TG-DTA) and Fourier transform infrared spectrometer (FTIR) measurements have been performed for pre- and post-fired sodium hydride (NaH) in the temperature range of 500-700 K, respectively. Temperature dependence of NaH thermal decomposition rates obtained by the isothermal TGs showed an inflection point at around 620 K, which was caused by two kinds of hydrogen states (rapid diffusing and immobile hydrogen). In the FTIR spectra for the NaH and sodium (Na), the specific signals were observed at around 873.4, 1010.4, 1049.5 and 1125.7 cm$$^{-1}$$, and the integrated values of FTIR signals for post-fired NaH at below 550K and at above 698 K were comparable to those for pre-fired NaH and Na, respectively. Those for post-fired NaH at 602-667 K were the intermediate values of the pre-fired NaH and Na, which denoted that the Na-Na bonds haven't grown sufficiently and the hydrogen coexisted in metallic Na. In order to predict the practical kinetics of NaH thermal decomposition reaction, we suggested the simple kinetics model which assumed two kinds of rapidly diffusing and immobile hydrogen states. The simulation results revealed the inflection point in temperature dependence of the thermal decomposition rates accordingly because the transition from immobile hydrogen to rapid diffusing hydrogen crosses over at around 620 K.

JAEA Reports

Development of technology for rapid analysis of strontium-90 with low isotopic abundance using laser resonance ionization (Contract research); FY2019 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; The University of Tokyo*

JAEA-Review 2020-024, 75 Pages, 2021/01

JAEA-Review-2020-024.pdf:5.43MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2019. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2018, this report summarizes the research results of the "Development of Technology for Rapid Analysis of Strontium-90 with Low Isotopic Abundance using Laser Resonance Ionization" conducted in FY2019. In this study, we will develop a rapid analysis technique for strontium-90 using diode laser-based resonance ionization with elemental and isotopic selectivity. Strontium-90 is one of the major difficult-to-measure nuclides released into the environment due to the accident at TEPCO's Fukushima Daiichi Nuclear Power Station. Our method is particularly intended for real samples which contain high concentrations of strontium stable isotopes such as marine samples.

Journal Articles

Improvement of adsorption performances of Sr adsorption fiber and investigation for realizing simple $$^{90}$$Sr analysis

Horita, Takuma; Asai, Shiho*; Konda, Miki; Matsueda, Makoto; Hanzawa, Yukiko; Kitatsuji, Yoshihiro

Bunseki Kagaku, 69(10/11), p.619 - 626, 2020/10

 Times Cited Count:0 Percentile:0(Chemistry, Analytical)

We have developed a Sr adsorption fiber for rapid analysis of $$^{90}$$Sr. The prepared Sr adsorption fiber has a Sr-extraction layer that densely retains a Sr-selective extractant, an 18-crown-6 ether derivative, on the fiber surface. Hydrophobic group-containing polymer chains embedded onto the surface of the fiber allow to form a hydrophobic phase, incorporating Sr-selective extractants. This unique surface structure provides high adsorption capacity, leading to rapid and highly efficient adsorption of Sr$$^{2+}$$. The adsorption capacity of the Sr adsorption fiber was 3 times higher than commercially available 18-crown-6 ether derivative-impregnated resin (Sr Resin). The equilibrium adsorption capacity of the Sr adsorption fiber was comparable to the Sr Resin. The retained $$^{90}$$Sr was finally determined by a GM counter. The total analysis time including the Sr adsorption and measurement was about 1 hour.

JAEA Reports

Assessment of the probability of aircraft crashing for HTTR

Ono, Masato; Hanawa, Yoshio; Sonobe, Hiroshi; Nishimura, Arashi; Sugaya, Naoto; Iigaki, Kazuhiko

JAEA-Technology 2020-010, 14 Pages, 2020/09

JAEA-Technology-2020-010.pdf:1.74MB

In response to new standard for regulating research and test reactor which is enforced December 18, 2013, it was carried out assessment of the probability of aircraft crashing for HTTR. According to assessment method provided in the Assessment Criteria of the Probability of Aircraft Crashing on Commercial Power Reactor Facilities, assessment was conducted targeting reactor building, spent fuel storage building and cooling tower. As a result, it was confirmed that the probability was 5.98$$times$$10$$^{-8}$$, which is lower than the assessment criteria 10$$^{-7}$$.

Journal Articles

A Large area position-sensitive scintillation neutron detector for upgrading SENJU diffractometer

Nakamura, Tatsuya; To, Kentaro; Ebine, Masumi; Birumachi, Atsushi; Sakasai, Kaoru

Proceedings of 2019 IEEE Nuclear Science Symposium and Medical Imaging Conference (NSS/MIC 2019), Vol.1, p.735 - 736, 2020/08

 Times Cited Count:0 Percentile:0.08(Nuclear Science & Technology)

A large area, position-sensitive scintillation neutron detector was developed for upgrading the SENJU, time-of-flight Laue single crystal neutron diffractometer, in J-PARC MLF. The detector has a neutron-sensitive area of 512 $$times$$ 512 mm with a pixel size of 4 $$times$$ 4 mm. The detector was developed for upgrading of the SENJU instrument. The large area detector is to be installed below the vacuum tank to enlarge a covering solid angle. A $$^{6}$$Li:ZnS (Ag) scintillator and wavelength-shifting fiber technologies are employed. Each fiber channel is read out individually with photon counting mode. The electronics boards are implemented at the backside of the detector, enabling the detector depth as short as 20 cm. The detector exhibited a detection efficiency of 45% for thermal neutron. No degradation in fiber position and in neutron sensitivity has been observed over one year after production. In this paper, detector design and detector performances are presented.

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